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Be true to your linework.
When you simplify the shading by using big and flat black areas, stay true to your descision and use big and flat colour areas also.
The linework is brilliant and has every information needed for the viewer to get the lighting and to feel that it is plastic,... so go for simple but expressive colouring.
First think of the colour and brightness of the lighted areas. What kinda light hits what kinda surface?
Try flat colouring and some well placed gradient fills, you may not feel something missing. For reference check Hellboy comics or 100Bullets...
If you want to model anything with colour, restrict yourself to use only one or two additional shades for each colour. And stay true to the hardedge black shadows by using only hardedge shades. For reference check the batman animated series (the bruce timm stuff).
example:
[link]
by the way do a colourstudy with a proper background and at least two or three different colours. not only skintone and white...
cheers
anjin
Thanks again.